Variations in cloud concentration nuclei related to continental air pollution control and maritime fuel regulation over the northwest Pacific Ocean
编号:1241 访问权限:仅限参会人 更新:2025-01-01 01:07:57 浏览:184次 口头报告

报告开始:2025年01月14日 13:45(Asia/Shanghai)

报告时间:15min

所在会场:[S25] Session 25-IGAC-SOLAS: Chemistry and Physics at Surface Ocean and Lower Atmosphere [S25-2] IGAC-SOLAS: Chemistry and Physics at Surface Ocean and Lower Atmosphere

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摘要
Here, we compared the concentrations of cloud condensation nuclei (CCN) and particle number size distributions (PNSDs) measured during the transient period from the winter to the summer East Asian monsoon in 2021 with those in 2014 to explore possible responses to how CCN responds to upwind continental air pollutant mitigation and marine traffic fuel sulfur content (FSC) regulation over the northwest Pacific Ocean (NWPO). We also employed the Positive Matrix Factorization (PMF) analysis to apportion concentrations of CCN (Nccn) to different sources in order to quantify its source-specified responses to mitigation of air pollution during the transient period. Our results showed that (1) upwind continental mitigation likely reduced Nccn by approximately 200 cm−3 and 400 cm−3 at 0.2% and 0.4% supersaturation (SS), respectively, in the marine background atmosphere over the NWPO; (2) FSC regulation resulted in a decrease in Nccn at 0.4% SS by about 50 cm−3 and was nearly negligible at 0.2% SS over the NWPO. Additionally, a PMF-resolved factor, characterized by a dominant nucleation mode, was present only in 2014 and disappeared in 2021, likely due to the reduction. This estimation, however, suffered from uncertainties since seasonal changes were hard to be deducted accurately. PMF-resolved factors accurately represented Nccn in 80–90% of cases, but this accuracy was not observed in the remaining cases. Finally, an integrated analysis of satellite-derived cloud parameters and ship-based measurements indicated that the reduced Nccn over the NWPO might be co-limited with meteorological factors in forming cloud droplets during the transient period.
关键词
cloud condensation nuclei, air pollutant mitigation, marine traffics, source apportionment, secondary aerosols
报告人
Xiaohong Yao
Professor Ocean University of China;Frontiers Science Center for Deep Ocean Multispheres and Earth System;Laboratory for Marine Ecology and Environmental Sciences

稿件作者
Xiaohong Yao Ocean University of China;Frontiers Science Center for Deep Ocean Multispheres and Earth System;Laboratory for Marine Ecology and Environmental Sciences
Lei Sun Ocean University of China
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重要日期
  • 会议日期

    01月13日

    2025

    01月17日

    2025

  • 09月27日 2024

    初稿截稿日期

  • 01月17日 2025

    注册截止日期

主办单位
State Key Laboratory of Marine Environmental Science, Xiamen University
承办单位
State Key Laboratory of Marine Environmental Science, Xiamen University
Department of Earth Sciences, National Natural Science Foundation of China
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